<?xml version="1.0" encoding="utf-8"?>
<XML>
	<ISCJOURNAL>
		<YEAR>2023</YEAR>
		<VOL>5</VOL>
		<NO>15</NO>
		<MOSALSAL>15</MOSALSAL>
		<PAGE_NO>15</PAGE_NO>
		<ARTICLES>
			<ARTICLE>
				<TitleF />
				<TitleE>Photodegradation of Ciprofloxacin, Acetaminophen, and Carbamazepine using g-C3N4-based materials for water treatment</TitleE>
				<TitleLang_ID>en</TitleLang_ID>
				<DOI>10.61186/jcc.5.2.6</DOI>
				<ABSTRACTS>
					<ABSTRACT>
						<Language_ID>en</Language_ID>
						<CONTENT>Recently, the use of photocatalytic materials has been suggested as a possible method for cleaning up the environment. A new photocatalyst for enhanced oxidation processes based on radicals is graphitic carbon nitride (g-C3N4), it is metal-free. g-C3N4 is a trendy two-dimensional (2D) photocatalyst with a number of advantages, such as responsiveness to strong stability, low cost, and visible light. In the present review, the synthesis and characterization of g-C3N4-based photocatalysts are discussed, along with some of their delegate applications in the treatment of wastewater and water (such as acetaminophen, ciprofloxacin, and carbamazepine removal). Meanwhile, the various methods of modification, including doping, defect introduction, heterojunctions, nanocomposites, and so on, are briefly discussed. The associated mechanisms and pertinent discoveries are also examined. Finally, the difficulties, the need for additional study, and the use of g-C3N4-based hybrid membranes are underlined.</CONTENT>
					</ABSTRACT>
				</ABSTRACTS>
				<PAGES>
					<PAGE>
						<FPAGE>125</FPAGE>
						<TPAGE>139</TPAGE>
					</PAGE>
				</PAGES>
				<AUTHORS>
					<AUTHOR>
						<NameE>Sogand</NameE>
						<MidNameE />
						<FamilyE>Bahadori</FamilyE>
						<Organizations>
							<Organization>Department of Chemistry, Kerman Branch, Islamic Azad University</Organization>
						</Organizations>
						<Countries>
							<Country>Iran</Country>
						</Countries>
						<EMAILS>
							<Email>Sogolbahadori@gmail.com</Email>
						</EMAILS>
					</AUTHOR>
					<AUTHOR>
						<NameE>Mohammadjavad</NameE>
						<MidNameE />
						<FamilyE>Sharifianjazi</FamilyE>
						<Organizations>
							<Organization>Department of Material Engineering, Isfahan University of Technology</Organization>
						</Organizations>
						<Countries>
							<Country>Iran</Country>
						</Countries>
						<EMAILS>
							<Email>mjsharifiancom877@gmail.com</Email>
						</EMAILS>
					</AUTHOR>
					<AUTHOR>
						<NameE>Sara</NameE>
						<MidNameE />
						<FamilyE>Eskandarinezhad</FamilyE>
						<Organizations>
							<Organization>Department of Mining and Metallurgy, Yazd University</Organization>
						</Organizations>
						<Countries>
							<Country>Iran</Country>
						</Countries>
						<EMAILS>
							<Email>s.eskandari.nezhad@gmail.com</Email>
						</EMAILS>
					</AUTHOR>
				</AUTHORS>
				<KEYWORDS>
					<KEYWORD>
						<KeyText>Photocatalyst degradation</KeyText>
					</KEYWORD>
					<KEYWORD>
						<KeyText>Photocatalyst</KeyText>
					</KEYWORD>
					<KEYWORD>
						<KeyText>g-C3N4</KeyText>
					</KEYWORD>
					<KEYWORD>
						<KeyText>Ciprofloxacin</KeyText>
					</KEYWORD>
					<KEYWORD>
						<KeyText>Acetaminophen</KeyText>
					</KEYWORD>
					<KEYWORD>
						<KeyText>Carbamazepine</KeyText>
					</KEYWORD>
				</KEYWORDS>
				<PDFFileName>Article6.pdf</PDFFileName>
				<REFRENCES>
					<REFRENCE>
						<REF>[1] J. Yu, M. Jaroniec, C. Jiang, Surface science of photocatalysis, Academic Press 2020.##[2] C. Bie, H. Yu, B. Cheng, W. Ho, J. Fan, J. Yu, Design, fabrication, and mechanism of nitrogen‐doped graphene‐based photocatalyst, Advanced Materials 33(9) (2021) 2003521.##[3] O.K. Dalrymple, E. Stefanakos, M.A. Trotz, D.Y. Goswami, A review of the mechanisms and modeling of photocatalytic disinfection, Applied Catalysis B: Environmental 98(1-2) (2010) 27-38.##[4] L. Zhang, X. Zhou, S. Liu, H. Liu, S. Zhu, Y. Mao, Q. Yang, S. Zhu, C. Zhang, T. Wang, C. Wang, Two birds, one stone: Rational design of Bi-MOF/g-C₃N₄ photocatalyst for effective nitrogen fixation and pollutants degradation, Journal of Cleaner Production 425 (2023) 138912.##[5] R.R. Ikreedeegh, M. Tahir, A critical review in recent developments of metal-organic-frameworks (MOFs) with band engineering alteration for photocatalytic CO₂ reduction to solar fuels, Journal of CO₂ Utilization 43 (2021) 101381.##[6] A. Meng, L. Zhang, B. Cheng, J. Yu, Dual cocatalysts in TiO₂ photocatalysis, Advanced Materials 31(30) (2019) 1807660.##[7] T. Di, Q. Xu, W. Ho, H. Tang, Q. Xiang, J. Yu, Review on metal sulphide‐based Z‐scheme photocatalysts, ChemCatChem 11(5) (2019) 1394-1411.##[8] C. Cheng, B. He, J. Fan, B. Cheng, S. Cao, J. Yu, An inorganic/organic S‐ scheme heterojunction H₂‐production photocatalyst and its charge transfer mechanism, Advanced Materials 33(22) (2021) 2100317.##[9] P. Xia, M. Antonietti, B. Zhu, T. Heil, J. Yu, S. Cao, Designing defective crystalline carbon nitride to enable selective CO₂ photoreduction in the gas phase, Advanced Functional Materials 29(15) (2019) 1900093.##[10] Y. Yang, X. Li, C. Zhou, W. Xiong, G. Zeng, D. Huang, C. Zhang, W. Wang, B. Song, X. Tang, X. Li, H. Guo, Recent advances in application of graphitic carbon nitride-based catalysts for degrading organic contaminants in water through advanced oxidation processes beyond photocatalysis: A critical review, Water Research 184 (2020) 116200.##[11] H.A. Bicalho, J.L. Lopez, I. Binatti, P.F.R. Batista, J.D. Ardisson, R.R. Resende, E. Lorençon, Facile synthesis of highly dispersed Fe(II)-doped g-C₃N₄ and its application in Fenton-like catalysis, Molecular Catalysis 435 (2017) 156-165.##[12] C. Chen, M. Xie, L. Kong, W. Lu, Z. Feng, J. Zhan, Mn₃O₄ nanodots loaded g-C₃N₄ nanosheets for catalytic membrane degradation of organic contaminants, Journal of Hazardous Materials 390 (2020) 122146.##[13] D. Van Thuan, T.B.H. Nguyen, T.H. Pham, J. Kim, T.T. Hien Chu, M.V. Nguyen, K.D. Nguyen, W.A. Al-onazi, M.S. Elshikh, Photodegradation of ciprofloxacin antibiotic in water by using ZnO-doped g-C₃N₄ photocatalyst, Chemosphere 308 (2022) 136408.##[14] J. Fan, H. Qin, S. Jiang, Mn-doped g-C₃N₄ composite to activate peroxymonosulfate for acetaminophen degradation: The role of superoxide anion and singlet oxygen, Chemical Engineering Journal 359 (2019) 723-732.##[15] A. Kane, L. Chafiq, S. Dalhatou, P. Bonnet, M. Nasr, N. Gaillard, J.M.D. Dikdim, G. Monier, A.A. Assadi, H. Zeghioud, g-C₃N₄/TiO₂ S-scheme heterojunction photocatalyst with enhanced photocatalytic Carbamazepine degradation and mineralization, Journal of Photochemistry and Photobiology A: Chemistry 430 (2022) 113971.##[16] N.Q. Thang, A. Sabbah, L.-C. Chen, K.-H. Chen, C.M. Thi, P. Van Viet, High-efficient photocatalytic degradation of commercial drugs for pharmaceutical wastewater treatment prospects: a case study of Ag/g-C₃N₄/ZnO nanocomposite materials, Chemosphere 282 (2021) 130971.##[17] Z. Chen, S. Zhang, Y. Liu, N.S. Alharbi, S.O. Rabah, S. Wang, X. Wang, Synthesis and fabrication of g-C₃N₄-based materials and their application in elimination of pollutants, Science of The Total Environment 731 (2020) 139054.##[18] M. Raaja Rajeshwari, S. Kokilavani, S. Sudheer Khan, Recent developments in architecturing the g-C₃N₄ based nanostructured photocatalysts: Synthesis, modifications and applications in water treatment, Chemosphere 291 (2022) 132735.##[19] M. Ahmaruzzaman, S.R. Mishra, Photocatalytic performance of g-C₃N₄ based nanocomposites for effective degradation/removal of dyes from water and wastewater, Materials Research Bulletin 143 (2021) 111417.##[20] B. Zhu, B. Cheng, J. Fan, W. Ho, J. Yu, g‐C₃N₄‐based 2D/2D composite heterojunction photocatalyst, Small Structures 2(12) (2021) 2100086.##[21] M. Zhang, Y. Yang, X. An, L.-a. Hou, A critical review of g-C₃N₄-based photocatalytic membrane for water purification, Chemical Engineering Journal 412 (2021) 128663.##[22] A. Smýkalová, B. Sokolová, K. Foniok, V. Matějka, P. Praus, Photocatalytic Degradation of Selected Pharmaceuticals Using g-C₃N₄ and TiO₂ Nanomaterials, Nanomaterials 9(9) (2019) 1194.##[23] D. Fatta-Kassinos, S. Meric, A. Nikolaou, Pharmaceutical residues in environmental waters and wastewater: current state of knowledge and future research, Analytical and Bioanalytical Chemistry 399(1) (2011) 251-275.##[24] A.M.E. Khalil, F.A. Memon, T.A. Tabish, D. Salmon, S. Zhang, D. Butler, Nanostructured porous graphene for efficient removal of emerging contaminants (pharmaceuticals) from water, Chemical Engineering Journal 398 (2020) 125440.##[25] Y. Gong, M. Li, H. Li, Y. Wang, Graphitic carbon nitride polymers: promising catalysts or catalyst supports for heterogeneous oxidation and hydrogenation, Green Chemistry 17(2) (2015) 715-736.##[26] X. Wang, K. Maeda, A. Thomas, K. Takanabe, G. Xin, J.M. Carlsson, K. Domen, M. Antonietti, A metal-free polymeric photocatalyst for hydrogen production from water under visible light, Nature materials 8(1) (2009) 76-80.##[27] D.M. Teter, R.J. Hemley, Low-compressibility carbon nitrides, Science 271(5245) (1996) 53-55.##[28] A. Thomas, A. Fischer, F. Goettmann, M. Antonietti, J.-O. Müller, R. Schlögl, J.M. Carlsson, Graphitic carbon nitride materials: variation of structure and morphology and their use as metal-free catalysts, Journal of Materials chemistry A 18(41) (2008) 4893-4908.##[29] T. Sano, S. Tsutsui, K. Koike, T. Hirakawa, Y. Teramoto, N. Negishi, K. Takeuchi, Activation of graphitic carbon nitride (gC₃N₄) by alkaline hydrother mal treatment for photocatalytic NO oxidation in gas phase, Journal of Materials Chemistry A 1(21) (2013) 6489-6496.##[30] K. Yu, X. Hu, K. Yao, P. Luo, X. Wang, H. Wang, Preparation of an ultrathin 2D/2D rGO/gC₃N₄ nanocomposite with enhanced visible-light-driven photocatalytic performance, RSC advances 7(58) (2017) 36793-36799.##[31] X. Bai, L. Wang, R. Zong, Y. Zhu, Photocatalytic activity enhanced via g-C₃N₄ nanoplates to nanorods, The Journal of Physical Chemistry C 117(19) (2013) 9952-9961.##[32] J. Zhu, Y. Wei, W. Chen, Z. Zhao, A. Thomas, Graphitic carbon nitride as a metal-free catalyst for NO decomposition, Chemical communications 46(37) (2010) 6965-6967.##[33] S. Cao, J. Low, J. Yu, M. Jaroniec, Polymeric photocatalysts based on graphitic carbon nitride, Advanced Materials 27(13) (2015) 2150-2176.##[34] X. Li, G. Huang, X. Chen, J. Huang, M. Li, J. Yin, Y. Liang, Y. Yao, Y. Li, A review on graphitic carbon nitride (g-C₃N₄) based hybrid membranes for water and wastewater treatment, Science of The Total Environment 792 (2021) 148462.##[35] R. Kumar, A. Sudhaik, P. Raizada, V.-H. Nguyen, Q. Van Le, T. Ahamad, S. Thakur, C.M. Hussain, P. Singh, Integrating K and P co-doped g-C₃N₄ with ZnFe₂O₄ and graphene oxide for S-scheme-based enhanced adsorption coupled photocatalytic real wastewater treatment, Chemosphere 337 (2023) 139267.##[36] Q. Wang, Y. Li, F. Huang, S. Song, G. Ai, X. Xin, B. Zhao, Y. Zheng, Z. Zhang, Recent advances in g-C₃N₄-based materials and their application in energy and environmental sustainability, Molecules 28(1) (2023) 432.##[37] N.F. Moreira, M.J. Sampaio, A.R. Ribeiro, C.G. Silva, J.L. Faria, A.M. Silva, Metal-free g-C₃N₄ photocatalysis of organic micropollutants in urban wastewater under visible light, Applied Catalysis B: Environmental 248 (2019) 184-192.##[38] J. Pan, Y. Liu, W. Ou, S. Li, H. Li, J. Wang, C. Song, Y. Zheng, C. Li, The photocatalytic hydrogen evolution enhancement of the MoS₂ lamellas modified g-C₃N₄/SrTiO₃ core-shell heterojunction, Renewable Energy 161 (2020) 340-349.##[39] M. Inagaki, T. Tsumura, T. Kinumoto, M. Toyoda, Graphitic carbon nitrides (g-C₃N₄) with comparative discussion to carbon materials, Carbon 141 (2019) 580- 607.##[40] H. Tang, S. Chang, G. Tang, W. Liang, AgBr and g-C₃N₄ co-modified Ag₂CO₃ photocatalyst: a novel multi-heterostructured photocatalyst with enhanced photocatalytic activity, Applied Surface Science 391 (2017) 440-448.##[41] G. Wang, X. Li, P. Hao, W. Liu, H. Zhan, S. Bi, g-C₃N₄/Nitrogen-Doped Carbon Dot/Silver Nanoparticle-Based Ternary Photocatalyst for Water Pollutant Treatment, ACS Applied Nano Materials 6(7) (2023) 5747-5758.##[42] Y. Zhang, J. Liu, G. Wu, W. Chen, Porous graphitic carbon nitride synthesized via direct polymerization of urea for efficient sunlight-driven photocatalytic hydrogen production, Nanoscale 4(17) (2012) 5300-5303.##[43] H. Dong, X. Guo, C. Yang, Z. Ouyang, Synthesis of g-C₃N₄ by different precursors under burning explosion effect and its photocatalytic degradation for tylosin, Applied Catalysis B: Environmental 230 (2018) 65-76.##[44] Z. Zhao, Y. Ma, J. Fan, Y. Xue, H. Chang, Y. Masubuchi, S. Yin, Synthesis of graphitic carbon nitride from different precursors by fractional thermal polymerization method and their visible light induced photocatalytic activities, Journal of Alloys and Compounds 735 (2018) 1297-1305.##[45] W.-J. Ong, L.-L. Tan, Y.H. Ng, S.-T. Yong, S.-P. Chai, Graphitic carbon nitride (g-C₃N₄)-based photocatalysts for artificial photosynthesis and environmental remediation: are we a step closer to achieving sustainability?, Chemical reviews 116(12) (2016) 7159-7329.##[46] Z. Mo, X. She, Y. Li, L. Liu, L. Huang, Z. Chen, Q. Zhang, H. Xu, H. Li, Synthesis of gC₃N₄ at different temperatures for superior visible/UV photocatalytic performance and photoelectrochemical sensing of MB solution, RSC advances 5(123) (2015) 101552-101562.##[47] Q. Tay, P. Kanhere, C.F. Ng, S. Chen, S. Chakraborty, A.C.H. Huan, T.C. Sum, R. Ahuja, Z. Chen, Defect engineered g-C₃N₄ for efficient visible light photocatalytic hydrogen production, Chemistry of Materials 27(14) (2015) 4930-4933.##[48] J. Xu, M. Fujitsuka, S. Kim, Z. Wang, T. Majima, Unprecedented effect of CO₂ calcination atmosphere on photocatalytic H₂ production activity from water using g-C₃N₄ synthesized from triazole polymerization, Applied Catalysis B: Environmental 241 (2019) 141-148.##[49] I. Khan, M. Luo, S. Khan, H. Asghar, M. Saeed, S. Khan, A. Khan, M. Humayun, L. Guo, B. Shi, Green synthesis of SrO bridged LaFeO₃/g-C₃N₄ nanocomposites for CO₂ conversion and bisphenol A degradation with new insights into mechanism, Environmental Research 207 (2022) 112650.##[50] S. Zhang, Y. Liu, P. Gu, R. Ma, T. Wen, G. Zhao, L. Li, Y. Ai, C. Hu, X. Wang, Enhanced photodegradation of toxic organic pollutants using dual-oxygen-doped porous g-C₃N₄: Mechanism exploration from both experimental and DFT studies, Applied Catalysis B: Environmental 248 (2019) 1-10.##[51] B. Zhou, M. Waqas, B. Yang, K. Xiao, S. Wang, C. Zhu, J. Li, J. Zhang, Convenient one-step fabrication and morphology evolution of thin-shelled honeycomb-like structured g-C₃N₄ to significantly enhance photocatalytic hydrogen evolution, Applied Surface Science 506 (2020) 145004.##[52] S. Zhang, S. Song, P. Gu, R. Ma, D. Wei, G. Zhao, T. Wen, R. Jehan, B. Hu, X. Wang, Visible-light-driven activation of persulfate over cyano and hydroxyl group co-modified mesoporous gC₃N₄ for boosting bisphenol A degradation, Journal of Materials Chemistry A 7(10) (2019) 5552-5560.##[53] C. Prasad, H. Tang, Q. Liu, I. Bahadur, S. Karlapudi, Y.J.i.j.o.h.e. Jiang, A latest overview on photocatalytic application of g-C₃N₄ based nanostructured materials for hydrogen production, 45(1) (2020) 337-379.##[54] X. Wang, X. Li, J. Wang, H. Zhu, Recent advances in carbon nitride-based nanomaterials for the removal of heavy metal ions from aqueous solution, Journal of Inorganic Materials 35(3) (2020).##[55] C. Bhuvaneswari, S.G. Babu, Nanoarchitecture and surface engineering strategy for the construction of 3D hierarchical CuS-rGO/g-C₃N₄ nanostructure: An ultrasensitive and highly selective electrochemical sensor for the detection of furazolidone drug, Journal of Electroanalytical Chemistry 907 (2022) 116080.##[56] C. Li, Z. Sun, Y. Xue, G. Yao, S. Zheng, A facile synthesis of g-C₃N₄/TiO₂ hybrid photocatalysts by sol–gel method and its enhanced photodegradation towards methylene blue under visible light, Advanced Powder Technology 27(2) (2016) 330-337.##[57] X. Liu, N. Chen, Y. Li, D. Deng, X. Xing, Y. Wang, A general nonaqueous sol-gel route to g-C₃N₄-coupling photocatalysts: the case of Z-scheme g-C₃N₄/ TiO₂ with enhanced photodegradation toward RhB under visible-light, Scientific Reports 6(1) (2016) 39531.##[58] F. Chang, J. Zhang, Y. Xie, J. Chen, C. Li, J. Wang, J. Luo, B. Deng, X. Hu, Fabrication, characterization, and photocatalytic performance of exfoliated g-C₃N₄–TiO₂ hybrids, Applied Surface Science 311 (2014) 574-581.##[59] F. Deng, L. Zhao, X. Pei, X. Luo, S. Luo, Facile in situ hydrothermal synthesis of g-C₃N₄/SnS₂ composites with excellent visible-light photocatalytic activity, Materials Chemistry and Physics 189 (2017) 169-175.##[60] V. Harish, M. Ansari, D. Tewari, A.B. Yadav, N. Sharma, S. Bawarig, M.-L. García-Betancourt, A. Karatutlu, M. Bechelany, A. Barhoum, Cutting-edge advances in tailoring size, shape, and functionality of nanoparticles and nanostructures: A review, Journal of the Taiwan Institute of Chemical Engineers 149 (2023) 105010.##[61] N. Cheng, J. Tian, Q. Liu, C. Ge, A.H. Qusti, A.M. Asiri, A.O. Al-Youbi, X. Sun, interfaces, Au-nanoparticle-loaded graphitic carbon nitride nanosheets: green photocatalytic synthesis and application toward the degradation of organic pollutants, ACS Applied Materials and Interfaces 5(15) (2013) 6815-6819.##[62] J. Di, J. Xia, S. Yin, H. Xu, L. Xu, Y. Xu, M. He, H. Li, Preparation of spherelike gC₃N₄/BiOI photocatalysts via a reactable ionic liquid for visible-light-driven photocatalytic degradation of pollutants, Journal of Materials chemistry A 2(15) (2014) 5340-5351.##[63] Y. Zhang, Y. Xu, L. Gao, X. Liu, Y. Fu, C. Ma, Y. Ge, R. Cao, X. Zhang, O.A. Al-Hartomy, S. Wageh, A. Al-Ghamdi, H. Algarni, Z. Shi, H. Zhang, MXene-based mixed-dimensional Schottky heterojunction towards self-powered flexible high-performance photodetector, Materials Today Physics 21 (2021) 100479.##[64] S. Meng, Y. Cui, H. Wang, X. Zheng, X. Fu, S. Chen, Noble metal-free 0D–1D NiSₓ/CdS nanocomposites toward highly efficient photocatalytic contamination removal and hydrogen evolution under visible light, Dalton Transactions 47(36) (2018) 12671-12683.##[65] O.J. Ajala, J.O. Tijani, M.T. Bankole, A.S. Abdulkareem, A critical review on graphene oxide nanostructured material: Properties, Synthesis, characterization and application in water and wastewater treatment, Environmental Nanotechnology, Monitoring and Management 18 (2022) 100673.##[66] Z. Talebzadeh, M. Masjedi-Arani, O. Amiri, M. Salavati-Niasari, La2Sn2O7/g-C3N4 nanocomposites: Rapid and green sonochemical fabrication and photo-degradation performance for removal of dye contaminations, Ultrasonics Sonochemistry 77 (2021) 105678.##[67] M.A. Tekalgne, S.Y. Kim, Research progress and perspectives on photocatalysts based on the lead-free double halide perovskite, EES Catalysis (2024).##[68] M.S. Umekar, G.S. Bhusari, T. Bhoyar, V. Devthade, B.P. Kapgate, A.P. Potbhare, R.G. Chaudhary, A.A. Abdala, Graphitic carbon nitride-based photocatalysts for environmental remediation of organic pollutants, Current Nanoscience 19(2) (2023) 148-169.##[69] Y. Zhen, C. Yang, H. Shen, W. Xue, C. Gu, J. Feng, Y. Zhang, F. Fu, Y. Liang, Photocatalytic performance and mechanism insights of a S-scheme g-C₃N₄/ Bi₂MoO₆ heterostructure in phenol degradation and hydrogen evolution reactions under visible light, Physical Chemistry Chemical Physics 22(45) (2020) 26278- 26288.##[70] D. Zhu, Q. Zhou, Nitrogen doped g-C₃N₄ with the extremely narrow band gap for excellent photocatalytic activities under visible light, Applied Catalysis B: Environmental 281 (2021) 119474.##[71] R. Acharya, K. Parida, A review on TiO₂/g-C₃N₄ visible-light-responsive photocatalysts for sustainable energy generation and environmental remediation, Journal of Environmental Chemical Engineering 8(4) (2020) 103896.##[72] H. Zhang, L. Jia, P. Wu, R. Xu, J. He, W. Jiang, Improved H₂O₂ photogeneration by KOH-doped g-C₃N₄ under visible light irradiation due to synergistic effect of N defects and K modification, Applied Surface Science 527 (2020) 146584.##[73] H. Liu, J. Liang, J. Du, Q. Gao, S. Fu, L. Li, M. Hu, F. Zhao, J. Zhou, Promoting charge separation in dual defect mediated Z-scheme MoS2/g-C3N4 photocatalysts for enhanced photocatalytic degradation activity: synergistic effect insight, Colloids and Surfaces A: Physicochemical and Engineering Aspects 594 (2020) 124668.##[74] D. Wang, J. Chen, X. Gao, Y. Ao, P. Wang, Maximizing the utilization of photo-generated electrons and holes of g-C₃N₄ photocatalyst for harmful algae inactivation, Chemical Engineering Journal 431 (2022) 134105.##[75] A. Mehtab, S.M. Alshehri, T. Ahmad, Photocatalytic and photoelectrocatalytic water splitting by porous g-C₃N₄ nanosheets for hydrogen generation, ACS Applied Nano Materials 5(9) (2022) 12656-12665.##[76] P. Murugesan, J. Moses, C. Anandharamakrishnan, Photocatalytic disinfection efficiency of 2D structure graphitic carbon nitride-based nanocomposites: a review, Journal of Materials Science 54(19) (2019) 12206-12235.##[77] C. Zhang, Y. Li, D. Shuai, Y. Shen, W. Xiong, L. Wang, Graphitic carbon nitride (g-C₃N₄)-based photocatalysts for water disinfection and microbial control: A review, Chemosphere 214 (2019) 462-479.##[78] T. Lin, Z. Song, Y. Wu, L. Chen, S. Wang, F. Fu, L. Guo, Boron-and phenyl-codoped graphitic carbon nitride with greatly enhanced light responsive range for photocatalytic disinfection, Journal of Hazardous Materials 358 (2018) 62-68.##[79] J.H. Thurston, N.M. Hunter, K.A. Cornell, Preparation and characterization of photoactive antimicrobial graphitic carbon nitride (g-C₃N₄) films, RSC advances 6(48) (2016) 42240-42248.##[80] Z. Liu, J. Wang, B. Kong, Z. Liu, T.-t. Song, W. Wang, Evidence of direct Z-scheme triazine-based gC₃N₄/BiOI (001) heterostructures: a hybrid density functional investigation, Physical Chemistry Chemical Physics 25(1) (2023) 847-856.##[81] J. Zou, G. Liao, J. Jiang, Z. Xiong, S. Bai, H. Wang, P. Wu, P. Zhang, X. Li, In-situ construction of sulfur-doped g-C3N4/defective g-C3N4 isotype step-scheme heterojunction for boosting photocatalytic H2 evolution, Chinese Journal of Structural Chemistry 41(1) (2022) 2201025-2201033.##[82] P. Mandyal, A. Guleria, R. Sharma, S. Sambyal, A. Priye, B. Fang, P. Shandilya, Insight into the properties, morphologies and photocatalytic applications of S-scheme Bi2WO6, Journal of Environmental Chemical Engineering (2022) 108918.##[83] M. Muhyuddin, G. Tseberlidis, M. Acciarri, O. Lori, M. D’Arienzo, M. Cavallini, P. Atanassov, L. Elbaz, A. Lavacchi, C. Santoro, Molybdenum disulfide as hydrogen evolution catalyst: From atomistic to materials structure and electrocatalytic performance, Journal of Energy Chemistry (2023).##[84] M. Ismael, Environmental remediation and sustainable energy generation via photocatalytic technology using rare earth metals modified g-C3N4: A review, Journal of Alloys and Compounds 931 (2023) 167469.##[85] M. Jyothi, V. Nayak, K.R. Reddy, S. Naveen, A. Raghu, Non-metal (oxygen, sulphur, nitrogen, boron and phosphorus)-doped metal oxide hybrid nanostructures as highly efficient photocatalysts for water treatment and hydrogen generation, Nanophotocatalysis and Environmental Applications: Materials and Technology (2019) 83-105.##[86] C. Prasad, H. Tang, Q. Liu, I. Bahadur, S. Karlapudi, Y. Jiang, A latest overview on photocatalytic application of g-C3N4 based nanostructured materials for hydrogen production, international journal of hydrogen energy 45(1) (2020) 337- 379.##[87] X. Liu, L. Rao, Y. Yao, H. Chen, Phosphorus-doped carbon fibers as an efficient metal-free bifunctional catalyst for removing sulfamethoxazole and chromium (VI), Chemosphere 246 (2020) 125783.##[88] T. Zahra, K.S. Ahmad, C. Zequine, R.K. Gupta, A.G. Thomas, M.A. Malik, S.B. Jaffri, D. Ali, Electro-catalyst [ZrO2/ZnO/PdO]-NPs green functionalization: fabrication, characterization and water splitting potential assessment, International Journal of Hydrogen Energy 46(37) (2021) 19347-19362.##[89] N.A.R. Che Mohamad, F. Marques Mota, D.H. Kim, Photocatalytic and Photoelectrochemical Overall Water Splitting, Solar‐to‐Chemical Conversion: Photocatalytic and Photoelectrochemcial Processes (2021) 189-242.##[90] G. Dong, K. Zhao, L. Zhang, Carbon self-doping induced high electronic conductivity and photoreactivity of gC3N4, Chemical communications 48(49) (2012) 6178-6180.##[91] F. Dong, Y. Li, Z. Wang, W.-K. Ho, Enhanced visible light photocatalytic activity and oxidation ability of porous graphene-like g-C3N4 nanosheets via thermal exfoliation, Applied Surface Science 358 (2015) 393-403.##[92] F. Zuo, L. Wang, T. Wu, Z. Zhang, D. Borchardt, P. Feng, Self-doped Ti3+ enhanced photocatalyst for hydrogen production under visible light, Journal of the American Chemical Society 132(34) (2010) 11856-11857.##[93] A. Kumar, P. Raizada, P. Singh, R.V. Saini, A.K. Saini, A. Hosseini-Bandegharaei, Perspective and status of polymeric graphitic carbon nitride based Z-scheme photocatalytic systems for sustainable photocatalytic water purification, Chemical Engineering Journal 391 (2020) 123496.##[94] Y. Pang, Y. Li, G. Xu, Y. Hu, Z. Kou, Q. Feng, J. Lv, Y. Zhang, J. Wang, Y. Wu, Z-scheme carbon-bridged Bi2O3/TiO2 nanotube arrays to boost photoelectrochemical detection performance, Applied Catalysis B: Environmental 248 (2019) 255-263.##[95] J. Wu, Y. Zhang, T. Wang, Y. Xin, D. Ma, Au nanoparticles and graphene oxide co-loaded graphitic carbon nitride: Synthesis and photocatalytic application, Materials Research Bulletin 100 (2018) 282-288.##[96] C. Daulbayev, F. Sultanov, B. Bakbolat, O. Daulbayev, 0D, 1D and 2D nanomaterials for visible photoelectrochemical water splitting. A review, International Journal of Hydrogen Energy 45(58) (2020) 33325-33342.##[97] H. Zhang, Y. Tang, Z. Liu, Z. Zhu, X. Tang, Y. Wang, Study on optical properties of alkali metal doped g-C3N4 and their photocatalytic activity for reduction of CO 2, Chemical Physics Letters 751 (2020) 137467.##[98] S. Zhang, P. Gu, R. Ma, C. Luo, T. Wen, G. Zhao, W. Cheng, X. Wang, Recent developments in fabrication and structure regulation of visible-light-driven g-C3N4-based photocatalysts towards water purification: a critical review, Catalysis Today 335 (2019) 65-77.##[99] Q. Zhu, Y. Xuan, K. Zhang, K. Chang, Enhancing photocatalytic CO2 reduction performance of g-C3N4-based catalysts with non-noble plasmonic nanoparticles, Applied Catalysis B: Environmental 297 (2021) 120440.##[100] Y. Fu, T. Huang, L. Zhang, J. Zhu, X. Wang, Ag/gC3N4 catalyst with superior catalytic performance for the degradation of dyes: a borohydride-generated superoxide radical approach, Nanoscale 7(32) (2015) 13723-13733.##[101] S. Tonda, S. Kumar, V. Shanker, Surface plasmon resonance-induced photocatalysis by Au nanoparticles decorated mesoporous g-C3N4 nanosheets under direct sunlight irradiation, Materials Research Bulletin 75 (2016) 51-58.##[102] S. Zhang, B. Li, X. Wang, G. Zhao, B. Hu, Z. Lu, T. Wen, J. Chen, X. Wang, Recent developments of two-dimensional graphene-based composites in visible-light photocatalysis for eliminating persistent organic pollutants from wastewater, Chemical Engineering Journal 390 (2020) 124642.##[103] M.B. Gawande, A. Goswami, F.-X. Felpin, T. Asefa, X. Huang, R. Silva, X. Zou, R. Zboril, R.S. Varma, Cu and Cu-based nanoparticles: synthesis and applications in catalysis, Chemical Reviews 116(6) (2016) 3722-3811.##[104] Y. Liu, Y. Zheng, W. Zhang, Z. Peng, H. Xie, Y. Wang, X. Guo, M. Zhang, R. Li, Y. Huang, Template-free preparation of non-metal (B, P, S) doped g-C3N4 tubes with enhanced photocatalytic H2O2 generation, Journal of Materials Science and Technology 95 (2021) 127-135.##[105] M.S. Nasir, G. Yang, I. Ayub, S. Wang, W. Yan, In situ decoration of g-C3N4 quantum dots on 1D branched TiO2 loaded with plasmonic Au nanoparticles and improved the photocatalytic hydrogen evolution activity, Applied Surface Science 519 (2020) 146208.##[106] G. Xu, Y. Xu, Z. Zhou, Y. Bai, Facile hydrothermal preparation of graphitic carbon nitride supercell structures with enhanced photodegradation activity, Diamond and Related Materials 97 (2019) 107461.##[107] Q. Xie, W. He, S. Liu, C. Li, J. Zhang, P.K. Wong, Bifunctional S-scheme g-C3N4/Bi/BiVO4 hybrid photocatalysts toward artificial carbon cycling, Chinese Journal of Catalysis 41(1) (2020) 140-153.##[108] X. He, S. Bai, J. Jiang, W.-J. Ong, J. Peng, Z. Xiong, G. Liao, J. Zou, N. Li, Oxygen vacancy mediated step-scheme heterojunction of WO2. 9/g-C3N4 for efficient electrochemical sensing of 4-nitrophenol, Chemical Engineering Journal Advances 8 (2021) 100175.##[109] X. Zhu, Y. Wang, Y. Guo, J. Wan, Y. Yan, Y. Zhou, C. Sun, Environmental-friendly synthesis of heterojunction photocatalysts g-C3N4/BiPO4 with enhanced photocatalytic performance, Applied Surface Science 544 (2021) 148872.##[110] S. Patnaik, S. Martha, S. Acharya, K. Parida, An overview of the modification of g-C3N4 with high carbon containing materials for photocatalytic applications, Separation and Purification Technology 3(3) (2016) 336-347.##[111] J. Wen, J. Xie, X. Chen, X. Li, A review on g-C3N4-based photocatalysts, Applied Surface Science 391 (2017) 72-123.##[112] S. Kumar, S. Karthikeyan, A.F. Lee, g-C3N4-based nanomaterials for visible light-driven photocatalysis, Catalysts 8(2) (2018) 74.##[113] F. Pei, S. Feng, Y. Wu, X. Lv, H. Wang, S.-M. Chen, Q. Hao, Y. Cao, W. Lei, Z. Tong, Label-free photoelectrochemical immunosensor for aflatoxin B1 detection based on the Z-scheme heterojunction of g-C3N4/Au/WO3, Biosensors and Bioelectronics 189 (2021) 113373.##[114] L. Wang, Y. Li, P. Han, Electrospinning preparation of g-C3N4/Nb2O5 nanofibers heterojunction for enhanced photocatalytic degradation of organic pollutants in water, Scientific Reports 11(1) (2021) 22950.##[115] J. Ren, S. Lv, S. Wang, M. Bao, X. Zhang, Y. Gao, Y. Liu, Z. Zhang, L. Zeng, J. Ke, Construction of efficient g-C3N4/NH2-UiO-66 (Zr) heterojunction photocatalysts for wastewater purification, Separation and Purification Technology 274 (2021) 118973.##[116] J. Liao, W. Cui, J. Li, J. Sheng, H. Wang, P. Chen, G. Jiang, Z. Wang, F. Dong, Nitrogen defect structure and NO+ intermediate promoted photocatalytic NO removal on H2 treated g-C3N4, Chemical Engineering Journal 379 (2020) 122282.##[117] W.-D. Oh, L.-W. Lok, A. Veksha, A. Giannis, T.-T. Lim, Enhanced photocatalytic degradation of bisphenol A with Ag-decorated S-doped g-C3N4 under solar irradiation: performance and mechanistic studies, Chemical Engineering Journal 333 (2018) 739-749.##[118] L. Liu, J. Huang, H. Yu, J. Wan, L. Liu, K. Yi, W. Zhang, C. Zhang, Construction of MoO3 nanopaticles/g-C3N4 nanosheets 0D/2D heterojuntion photocatalysts for enhanced photocatalytic degradation of antibiotic pollutant, Chemosphere 282 (2021) 131049.##[119] P. Niu, L.C. Yin, Y.Q. Yang, G. Liu, H.M. Cheng, Increasing the visible light absorption of graphitic carbon nitride (Melon) photocatalysts by homogeneous self‐modification with nitrogen vacancies, Advanced Materials 26(47) (2014) 8046-8052.##[120] J. Wu, N. Li, H.-B. Fang, X. Li, Y.-Z. Zheng, X. Tao, Nitrogen vacancies modified graphitic carbon nitride: Scalable and one-step fabrication with efficient visible-light-driven hydrogen evolution, Chemical Engineering Journal 358 (2019) 20-29.##[121] J. Ding, W. Xu, H. Wan, D. Yuan, C. Chen, L. Wang, G. Guan, W.-L. Dai, Nitrogen vacancy engineered graphitic C3N4-based polymers for photocatalytic oxidation of aromatic alcohols to aldehydes, Applied Catalysis B: Environmental 221 (2018) 626-634.##[122] Z. Wang, Y. Huang, M. Chen, X. Shi, Y. Zhang, J. Cao, W. Ho, S.C. Lee, Roles of N-vacancies over porous g-C3N4 microtubes during photocatalytic NOx removal, ACS Applied Materials and Interfaces 11(11) (2019) 10651-10662.##[123] D. Chen, J. Yang, H. Ding, Synthesis of nanoporous carbon nitride using calcium carbonate as templates with enhanced visible-light photocatalytic activity, Applied Surface Science 391 (2017) 384-391.##[124] Y. Yang, L. Geng, Y. Guo, J. Meng, Y. Guo, Easy dispersion and excellent visible-light photocatalytic activity of the ultrathin urea-derived g-C3N4 nanosheets, Applied Surface Science 425 (2017) 535-546.##[125] X. Wang, Q. Liu, Q. Yang, Z. Zhang, X. Fang, Three-dimensional g-C3N4 aggregates of hollow bubbles with high photocatalytic degradation of tetracycline, Carbon 136 (2018) 103-112.##[126] Z. Jin, Q. Zhang, S. Yuan, T. Ohno, Synthesis high specific surface area nanotube gC3N4 with two-step condensation treatment of melamine to enhance photocatalysis properties, Rsc Advances 5(6) (2015) 4026-4029.##[127] C. Fan, Q. Feng, G. Xu, J. Lv, Y. Zhang, J. Liu, Y. Qin, Y. Wu, Enhanced photocatalytic performances of ultrafine g-C3N4 nanosheets obtained by gaseous stripping with wet nitrogen, Applied Surface Science 427 (2018) 730-738.##[128] T. Yu, T. Xie, W. Zhou, Y. Zhang, Y. Chen, B. Shao, W.-Q. Guo, X. Tan, Fumaric acid assistant band structure tunable nitrogen defective g-C3N4 fabrication for enhanced photocatalytic hydrogen evolution, ACS Sustainable Chemistry and Engineering 9(22) (2021) 7529-7540.##[129] Y. Qin, J. Lu, X. Zhao, X. Lin, Y. Hao, P. Huo, M. Meng, Y. Yan, Nitrogen defect engineering and π-conjugation structure decorated g-C3N4 with highly enhanced visible-light photocatalytic hydrogen evolution and mechanism insight, Chemical Engineering Journal 425 (2021) 131844.##[130] A. Torres-Pinto, A.M. Díez, C.G. Silva, J.L. Faria, M.Á. Sanromán, A.M. Silva, M. Pazos, Photoelectrocatalytic degradation of pharmaceuticals promoted by a metal-free gC3N4 catalyst, Chemical Engineering Journal 476 (2023) 146761.##[131] A. Balakrishnan, M. Chinthala, R.K. Polagani, D.-V.N. Vo, Removal of tetracycline from wastewater using g-C3N4 based photocatalysts: A review, Environmental Research 216 (2023) 114660.##[132] D. Ramírez-Morales, M. Masís-Mora, J.R. Montiel-Mora, M. Méndez-Rivera, J.A. Gutiérrez-Quirós, L. Brenes-Alfaro, C.E. Rodríguez-Rodríguez, Pharmaceuticals, hazard and ecotoxicity in surface and wastewater in a tropical dairy production area in Latin America, Chemosphere (2023) 140443.##[133] G.Z.S. Ling, S.F. Ng, W.J. Ong, Tailor‐engineered 2D cocatalysts: harnessing electron–hole redox center of 2D g‐C3N4 photocatalysts toward solar‐to‐chemical conversion and environmental purification, Advanced Functional Materials 32(29) (2022) 2111875.##[134] P. Gan, Y. Lu, Y. Li, W. Liu, L. Chen, M. Tong, J. Liang, Non-radical degradation of organic pharmaceuticals by g-C3N4 under visible light irradiation: The overlooked role of excitonic energy transfer, Journal of Hazardous Materials 445 (2023) 130549.##[135] J. Rashid, A. Abbas, L.C. Chang, A. Iqbal, I.U. Haq, A. Rehman, S.U. Awan, M. Arshad, M. Rafique, M. Barakat, Butterfly cluster like lamellar BiOBr/TiO2 nanocomposite for enhanced sunlight photocatalytic mineralization of aqueous ciprofloxacin, Science of the Total Environment 665 (2019) 668-677.##[136] Y. Zhou, L. Zhou, C. Ni, E. He, L. Yu, X. Li, 3D/2D MOF-derived CoCeOx/g-C3N4 Z-scheme heterojunction for visible light photocatalysis: Hydrogen production and degradation of carbamazepine, Journal of Alloys and Compounds 890 (2022) 161786.##[137] E. Cako, S. Dudziak, P. Głuchowski, G. Trykowski, M. Pisarek, A.F. Borzyszkowska, K. Sikora, A. Zielińska-Jurek, Heterojunction of (P, S) co-doped g-C3N4 and 2D TiO2 for improved carbamazepine and acetaminophen photocatalytic degradation, Separation and Purification Technology 311 (2023) 123320.##[138] E.S. Okeke, K.I. Chukwudozie, R. Nyaruaba, R.E. Ita, A. Oladipo, O. Ejeromedoghene, E.O. Atakpa, C.V. Agu, C.O. Okoye, Antibiotic resistance in aquaculture and aquatic organisms: a review of current nanotechnology applications for sustainable management, Environmental Science and Pollution Research 29(46) (2022) 69241-69274.##[139] X. Yang, Z. Chen, W. Zhao, C. Liu, X. Qian, M. Zhang, G. Wei, E. Khan, Y.H. Ng, Y.S. Ok, Recent advances in photodegradation of antibiotic residues in water, Chemical Engineering Journal 405 (2021) 126806.##[140] S.K. Fanourakis, J. Peña-Bahamonde, P.C. Bandara, D.F. Rodrigues, Nano-based adsorbent and photocatalyst use for pharmaceutical contaminant removal during indirect potable water reuse, NPJ Clean Water 3(1) (2020) 1.##[141] Y. Liu, X. Zeng, X. Hu, J. Hu, Z. Wang, Y. Yin, C. Sun, X. Zhang, Two-dimensional g-C3N4/TiO2 nanocomposites as vertical Z-scheme heterojunction for improved photocatalytic water disinfection, Catalysis Today 335 (2019) 243-251.##[142] H. Zhang, W. Wu, Y. Li, Y. Wang, C. Zhang, W. Zhang, L. Wang, L. Niu, Enhanced photocatalytic degradation of ciprofloxacin using novel C-dot@ Nitrogen deficient g-C3N4: synergistic effect of nitrogen defects and C-dots, Applied Surface Science 465 (2019) 450-458.##[143] H. Li, Y. Gao, X. Wu, P.-H. Lee, K. Shih, Fabrication of heterostructured g-C3N4/Ag-TiO2 hybrid photocatalyst with enhanced performance in photocatalytic conversion of CO 2 under simulated sunlight irradiation, Applied Surface Science 402 (2017) 198-207.##[144] H. Liang, J. Guo, M. Yu, Y. Zhou, R. Zhan, C. Liu, J. Niu, Porous loofah-sponge-like ternary heterojunction g-C3N4/Bi2WO6/MoS2 for highly efficient photocatalytic degradation of sulfamethoxazole under visible-light irradiation, Chemosphere 279 (2021) 130552.##[145] N. Lu, P. Wang, Y. Su, H. Yu, N. Liu, X. Quan, Construction of Z-Scheme g-C3N4/RGO/WO3 with in situ photoreduced graphene oxide as electron mediator for efficient photocatalytic degradation of ciprofloxacin, Chemosphere 215 (2019) 444-453.##[146] J. Huang, W. Chen, X. Yu, X. Fu, Y. Zhu, Y. Zhang, Fabrication of a ternary BiOCl/CQDs/rGO photocatalyst: The roles of CQDs and rGO in adsorption-photocatalytic removal of ciprofloxacin, Colloids and Surfaces A: Physicochemical and Engineering Aspects 597 (2020) 124758.##[147] N. Roy, S.A. Alex, N. Chandrasekaran, A. Mukherjee, K. Kannabiran, A comprehensive update on antibiotics as an emerging water pollutant and their removal using nano-structured photocatalysts, Journal of Environmental Chemical Engineering 9(2) (2021) 104796.##[148] M. Verma, A. Haritash, Photocatalytic degradation of Amoxicillin in pharmaceutical wastewater: A potential tool to manage residual antibiotics, Environmental Technology and Innovation 20 (2020) 101072.##[149] S. Shenoy, C. Chuaicham, T. Okumura, K. Sekar, K. Sasaki, Simple tactic polycondensation synthesis of Z-scheme quasi-polymeric g-C3N4/CaFe2O4 composite for enhanced photocatalytic water depollution via pn heterojunction, Chemical Engineering Journal 453 (2023) 139758.##[150] Z. Hu, X. Cai, Z. Wang, S. Li, Z. Wang, X. Xie, Construction of carbon-doped supramolecule-based g-C3N4/TiO2 composites for removal of diclofenac and carbamazepine: A comparative study of operating parameters, mechanisms, degradation pathways, Journal of hazardous materials 380 (2019) 120812.##[151] X. Wang, P. Zhang, L. Li, N. Li, X. Su, X. Wei, L. Han, Preparation of a high-performance N-defect ZnO@ g-C3N4 nanocomposite and its photocatalytic degradation of tetracycline, Materials Today Communications 36 (2023) 106732.##[152] M. Yu, H. Liang, R. Zhan, L. Xu, J. Niu, Sm-doped g-C3N4/Ti3C2 MXene heterojunction for visible-light photocatalytic degradation of ciprofloxacin, Chinese Chemical Letters 32(7) (2021) 2155-2158.##[153] I. Ihsanullah, MXenes as next-generation materials for the photocatalytic degradation of pharmaceuticals in water, Journal of Environmental Chemical Engineering 10(3) (2022) 107381.##[154] S. Lu, C. Li, H. Li, Y. Zhao, Y. Gong, L. Niu, X. Liu, T. Wang, The effects of nonmetal dopants on the electronic, optical and chemical performances of monolayer g–C3N4 by first-principles study, Applied Surface Science 392 (2017) 966-974.##[155] K. Hu, R. Li, C. Ye, A. Wang, W. Wei, D. Hu, R. Qiu, K. Yan, Facile synthesis of Z-scheme composite of TiO2 nanorod/g-C3N4 nanosheet efficient for photocatalytic degradation of ciprofloxacin, Journal of Cleaner Production 253 (2020) 120055.##[156] L.K.B. Paragas, V. Dien Dang, R.S. Sahu, S. Garcia-Segura, M.D.G. de Luna, J.A.I. Pimentel, R.-A. Doong, Enhanced visible-light-driven photocatalytic degradation of acetaminophen over CeO2/I, K-codoped C3N4 heterojunction with tunable properties in simulated water matrix, Separation and Purification Technology 272 (2021) 117567.##[157] H.N. Phong Vo, G.K. Le, T.M. Hong Nguyen, X.-T. Bui, K.H. Nguyen, E.R. Rene, T.D.H. Vo, N.-D. Thanh Cao, R. Mohan, Acetaminophen micropollutant: Historical and current occurrences, toxicity, removal strategies and transformation pathways in different environments, Chemosphere 236 (2019) 124391.##[158] E. Brillas, J. Manuel Peralta-Hernández, Removal of paracetamol (acetaminophen) by photocatalysis and photoelectrocatalysis. A critical review, Separation and Purification Technology 309 (2023) 122982.##[159] M. Noorisepehr, B. Kakavandi, A.A. Isari, F. Ghanbari, E. Dehghanifard, N. Ghomi, F. Kamrani, Sulfate radical-based oxidative degradation of acetaminophen over an efficient hybrid system: Peroxydisulfate decomposed by ferroferric oxide nanocatalyst anchored on activated carbon and UV light, Separation and Purification Technology 250 (2020) 116950.##[160] K. Li, J. Chen, Y. Ao, P. Wang, Preparation of a ternary g-C3N4-CdS/Bi4O5I2 composite photocatalysts with two charge transfer pathways for efficient degradation of acetaminophen under visible light irradiation, Separation and Purification Technology 259 (2021) 118177.##[161] S. Moradi, A.A. Isari, F. Hayati, R. Rezaei Kalantary, B. Kakavandi, Co-implanting of TiO2 and liquid-phase-delaminated g-C3N4 on multi-functional graphene nanobridges for enhancing photocatalytic degradation of acetaminophen, Chemical Engineering Journal 414 (2021) 128618.##[162] S. Gupta, J. Gandhi, S. Kokate, L.G. Raikar, V.G. Kopuri, H. Prakash, Augmented photocatalytic degradation of Acetaminophen using hydrothermally treated g-C3N4 and persulfate under LED irradiation, Heliyon 9(5) (2023).##[163] F.J. Benitez, J.L. Acero, F.J. Real, G. Roldan, E. Rodriguez, Photolysis of model emerging contaminants in ultra-pure water: Kinetics, by-products formation and degradation pathways, Water Research 47(2) (2013) 870-880.##[164] K. Perović, F.M. dela Rosa, M. Kovačić, H. Kušić, U.L. Štangar, F. Fresno, D.D. Dionysiou, A. Loncaric Bozic, Recent Achievements in Development of TiO 2-Based Composite Photocatalytic Materials for Solar Driven Water Purification and Water Splitting, Materials 13(6) (2020) 1338.##[165] A. Hayat, J.A. Shah Syed, A.G. Al-Sehemi, K.S. El-Nasser, T.A. Taha, A.A. Al-Ghamdi, M.A. Amin, Z. Ajmal, W. Iqbal, A. Palamanit, D.I. Medina, W.I. Nawawi, M. Sohail, State of the art advancement in rational design of g-C3N4 photocatalyst for efficient solar fuel transformation, environmental decontamination and future perspectives, International Journal of Hydrogen Energy 47(20) (2022) 10837-10867.##[166] M. Israel, P. Beaudry, Carbamazepine in Psychiatry: A Review, The Canadian Journal of Psychiatry 33(7) (1988) 577-584.##[167] K. Chojnacka, D. Skrzypczak, G. Izydorczyk, K. Mikula, D. Szopa, K. Moustakas, A. Witek-Krowiak, Biodegradation of pharmaceuticals in photobioreactors – a systematic literature review, Bioengineered 13(2) (2022) 4537-4556.##[168] M.N. Chong, B. Jin, G. Laera, C.P. Saint, Evaluating the photodegradation of Carbamazepine in a sequential batch photoreactor system: Impacts of effluent organic matter and inorganic ions, Chemical Engineering Journal 174(2) (2011) 595-602.##[169] Y. Zhang, S.-U. Geißen, C. Gal, Carbamazepine and diclofenac: Removal in wastewater treatment plants and occurrence in water bodies, Chemosphere 73(8) (2008) 1151-1161.##[170] A.S. Mestre, A.P. Carvalho, Photocatalytic Degradation of Pharmaceuticals Carbamazepine, Diclofenac, and Sulfamethoxazole by Semiconductor and Carbon Materials: A Review, Molecules 24(20) (2019) 3702.##[171] J. Deng, Y. Shao, N. Gao, S. Xia, C. Tan, S. Zhou, X. Hu, Degradation of the antiepileptic drug carbamazepine upon different UV-based advanced oxidation processes in water, Chemical Engineering Journal 222 (2013) 150-158.##[172] R. Kumar, M. Qureshi, D.K. Vishwakarma, N. Al-Ansari, A. Kuriqi, A. Elbeltagi, A. Saraswat, A review on emerging water contaminants and the application of sustainable removal technologies, Case Studies in Chemical and Environmental Engineering 6 (2022) 100219.##[173] P. Gan, Z. Zhang, Y. Hu, Y. Li, J. Ye, M. Tong, J. Liang, Insight into the role of Fe in the synergetic effect of persulfate/sulfite and Fe2O3@g-C3N4 for carbamazepine degradation, Science of The Total Environment 819 (2022) 152787.##[174] T. Xu, D. Wang, L. Dong, H. Shen, W. Lu, W. Chen, Graphitic carbon nitride co-modified by zinc phthalocyanine and graphene quantum dots for the efficient photocatalytic degradation of refractory contaminants, Applied Catalysis B: Environmental 244 (2019) 96-106.##[175] L. Yang, L. Liang, L. Wang, J. Zhu, S. Gao, X. Xia, Accelerated photocatalytic oxidation of carbamazepine by a novel 3D hierarchical protonated g-C3N4/ BiOBr heterojunction: Performance and mechanism, Applied Surface Science 473 (2019) 527-539.##[176] X. Mei, S. Chen, G. Wang, W. Chen, W. Lu, B. Zhang, Y. Fang, C. Qi, Metal-free carboxyl modified g-C3N4 for enhancing photocatalytic degradation activity of organic pollutants through peroxymonosulfate activation in wastewater under solar radiation, Journal of Solid State Chemistry 310 (2022) 123053.##[177] Z. Cheng, L. Ling, J. Fang, C. Shang, Visible light-driven g-C3N4 peroxymonosulfate activation process for carbamazepine degradation: Activation mechanism and matrix effects, Chemosphere 286 (2022) 131906.##[178] T. Xia, Q. Hou, H. Qian, R. Lai, X. Bai, G. Yu, W. Zhang, M.L.U. Rehman, M. Ju, Fabricating metal-free Z-scheme heterostructures with nitrogen-deficient carbon nitride for fast photocatalytic removal of acetaminophen, Separation and Purification Technology 308 (2023) 122964.##[179] X. Du, X. Bai, L. Xu, L. Yang, P. Jin, Visible-light activation of persulfate by TiO 2/g-C3N4 photocatalyst toward efficient degradation of micropollutants, Chemical Engineering Journal 384 (2020) 123245.##[180] F. Al Marzouqi, R. Selvaraj, Y. Kim, Rapid photocatalytic degradation of acetaminophen and levofloxacin using g-C3N4 nanosheets under solar light irradiation, Materials Research Express 6(12) (2020) 125538.##[181] A. Hassani, P. Eghbali, B. Kakavandi, K.-Y.A. Lin, F. Ghanbari, Acetaminophen removal from aqueous solutions through peroxymonosulfate activation by CoFe2O4/mp g-C3N4 nanocomposite: Insight into the performance and degradation kinetics, Environmental Technology and Innovation 20 (2020) 101127.##[182] W. Hou, C. Deng, H. Xu, D. Li, Z. Zou, H. Xia, D. Xia, n–p BiOCl@ g-C3N4 Heterostructure with Rich‐oxygen Vacancies for Photodegradation of Carbamazepine, ChemistrySelect 5(9) (2020) 2767-2777.##[183] F. Goudarzy, J. Zolgharnein, J.B. Ghasemi, Determination and degradation of carbamazepine using g-C3N4@ CuS nanocomposite as sensitive fluorescence sensor and efficient photocatalyst, Inorganic Chemistry Communications 141 (2022) 109512.##[184] N.S. Alhokbany, R. Mousa, M. Naushad, S.M. Alshehri, T. Ahamad, Fabrication of Z-scheme photocatalysts g-C3N4/Ag3PO4/chitosan for the photocatalytic degradation of ciprofloxacin, International Journal of Biological Macromolecules 164 (2020) 3864-3872.##[185] W. Shi, Y. Liu, W. Sun, Y. Hong, X. Li, X. Lin, F. Guo, J. Shi, Assembling g-C3N4 nanosheets on rod-like CoFe2O4 nanocrystals to boost photocatalytic degradation of ciprofloxacin with peroxymonosulfate activation, Materials Today Communications 29 (2021) 102871.##[186] H. Liang, M. Yu, J. Guo, R. Zhan, J. Chen, D. Li, L. Zhang, J. Niu, A novel vacancy-strengthened Z-scheme g-C3N4/Bp/MoS2 composite for super-efficient visible-light photocatalytic degradation of ciprofloxacin, Separation and Purification Technology 272 (2021) 118891.##[187] J. Zhou, B. Zhu, Novel 1D/3D CeO2/g-C3N4 catalysts for photodegradation of ciprofloxacin under visible light via dimensional regulation and heterostructure construction, Journal of Physics and Chemistry of Solids 171 (2022) 111002.</REF>
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